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마약길항제의 방출 제어형 제제 ( 제1보 ) : 생체분해성 polyphosphazenes의 합성과 나록손 이식제제의 제조 및 용출특성
Controlled Release Dosage Form of Narcotic Antagonist ( Ⅰ ) : Synthesis of Biodegradable Polyphosphazenes and Preparation and Release Characteristics of Naloxone Implant
박주애 , 이승진 , 김형국 , 김길수 ( Joo Ae Park , Seung Jin Lee , Hyug Kuk Kim , Kil Soo Kim )
약제학회지 25권 2호 109-116(8pages)
UCI I410-ECN-0102-2008-510-000814710

For the administration of narcotic antagonist with short half-life and low patient compliance, the sustained release system using biodegradable matrix is effective. Polyphosphazenes are of considerable interest as biodegradable matrix systems for controlled release of drugs. In this study, biodegradable polyphosphazenes available for the sustained release implantable device were synthesized, and their application was examined. Poly[dichlorophosphazene] was synthesized by solution polymerization method and confirmed with IR spectrum. Poly[bis(ethyl glycinate) phosphazene] and poly[(diethyl glutamate)-co-(ethyl glycinate)phosphazene] were then produced by substitution of amino acid alkyl esters for chloride side groups. Using these polymers, the implantable devices of 1 mm thickness and 10×10 mm size containing naloxone hydrochloride were prepared and their release and degradation profiles were measured. In the case of poly[bis(ethyl glycinate)phosphazene] with swelling characteristics, degradation rate was slower than the release rate, showing that the release rate is partly dependent on the swelling rate. In contrast, the degradation rate of poly[(diethyl glutamate)-co-(ethyl glycinate)phosphazene] matrix was identical with release rate of naloxone hydrochloride. On the basis of these results, it is expected that these polymers can be applied to sustained release implantable systems delivering narcotic antagonist.

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