18.97.14.84
18.97.14.84
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Monopyridinium Oxime 과 Bispyridinium Oxime 화합물의 수용액 중 안정성 연구
Stability of Mono - and Bis - pyridinium Oximes in Aqueous Systems
정창희(Chang - Hee Jung), 최승주(Seung - Ju Choi), 서원준(Won - Jun Seo), 석대은(Dai - Eun Sok)
UCI I410-ECN-0102-2008-510-000816118

The stability of three oximes, HI-6 [(4-carbamoyl-2`[(hydroxyimino)-methyl]- 1,1`-oxydimethylenedi-(pyridinium chloride)], HI-CN [(4 cyano-2`-[(hydroxyimino)-methyl]-1,1`-oxydimethylene-di-(pyridinium chloride)], and 2-PAM [pralidoxime chloride] in aqueous solutions was evaluated by HPLC assay. The rate of degradation is dependent on the pH as well as the temperature at which the solution is stored. The optimum pH for the stability of these oximes was pH 2 to 3. The degradation rate constant for 2-PAM (k at 70℃, 2.07×10^(-4)/hr; E_a value, 27.2 ㎉/㏖) was smaller than those for bis-pyridinium oximes, HI-6 (k at 70℃, 3.38×10^(-3)/hr) and HI-CN (k at 70℃, 8.66×10^(-3)/hr; Ea value, 20.7 ㎉/㏖). In mechanistic analyses, it was found that HI-CN was decomposed through not only the hydrolysis of nitrile group but also the cleavage of methylene ether bridge, in contrast to HI-6 which was degraded mainly through the cleavage of methylene ether bridge.

[자료제공 : 네이버학술정보]
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