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1,2-Bis(4-phenoxy)benzene 구조를 함유하는 신규의 용해성 방향족 Polyamide-imide의 합성과 성질
Preparation and Properties of Noble Aromatic Soluble Poly (amide-imide)s Containing 1,2-Bis(4-phenoxy)benzene Units
오예미 ( Yae Mi O ) , 정화진 ( Hwa Jin Jeong )
UCI I410-ECN-0102-2009-580-003878578
* 발행 기관의 요청으로 구매가 불가능한 자료입니다.

A new diimide-dicarboxylic acid, 1,2-bis(4-trimellitimidophenoxy)benzene[1,2-BTPB), having flexible 1,2-bis(4-phenoxy)benzene unit was synthesized by the condensation reaction of 1,2-bis(4-aminophenoxy)benzene with trimellitic anhydride in N,N-dimethylformamide (DMF). A series of new poly(amide-imide)s were prepared by direct polycondensation of 1,2-BTPB and aromatic diamines containing multiaromatic rings linked with various flexible or bulky linkages in N-methyl-2-pyrrolidone(NMP), using triphenyl phosphite and pyridine as condensing agents. The resultant polymers had moderate inherent viscosities of 0.31-0.78 dL/g and wide-angle X-ray diffractograms revealed that the polymers were amorphous. Most of polymers exhibited good solubility and could be readily dissolved in various solvents such as DMF, NMP, N,N-dimethylacetamide, N,N-dimethylsulfoxide, m-cresol, and pyridine. The glass transition temperatures of the polymers occurred over the temperature range of 213∼302℃ in their differential scanning calorimetry(DSC) curves and their 10% weight loss temperature in air and nitrogen were in the range of 485∼530 ℃ and 480∼550℃, respectively, by thermogravimetric analysis(TGA). All the polymers did not lose weight below 400℃ in air and nitrogen, and their DSC curves also revealed similar decomposition behavior to that of TGA with no transition below the decomposition temperatures.

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