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상이동 촉매를 이용한 고분자로의 이산화탄소 직접 고정화
Direct Incorporation of Carbon Dioxide to Polymer Using Phase Transfer Catalyst
성충기 , 김경훈 , 문정열 , 박대원 ( C . K . Sung , K . H . Kim , J . Y . Moon , D . W . Park )
응용화학 vol. 2 iss. 1 468-471(4pages)
UCI I410-ECN-0102-2009-570-007308242
This article is 4 pages or less.

This study is related to the investigation of the direct incorporation of CO₂ to polymer using phase transfer catalysts. Quaternary ammonium salts showed good catalytic activity of CO₂ fixation in the synthesis of poly(1,3-dioxolane-2-oxo-4-yl) methyl methacrylate by the direct incorporation of CO₂ to poly(GMA). Among the salts tested, the ones with higher alkyl chain length and with more nucleophilic anion showed higher catalytic activity. The catalytic activity increased with temperature and DMF showed the highest activity. Kinetic studies at high pressure of CO₂ were also investigated, and polymer-supported catalysts were used to facilitate the recovery of catalysts.

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